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There is a shuttle bus service that departs Nairobi at 08.00 and 14.00 daily to Arusha in Tanzania. Arrival in Arusha is at approx 13.00 and 19.00 respectively (about 5 hours if no hold-ups at the border – so you should allow 6 hours to be on safe side). They depart from Arusha to Nairobi also at 08.00 and 14.00 each day.
